Please use this identifier to cite or link to this item: https://hdl.handle.net/20.500.11851/4105
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dc.contributor.authorAltaf, Çiğdem Tuc-
dc.contributor.authorŞahsuvar, N. S.-
dc.contributor.authorAbdullayeva, N.-
dc.contributor.authorCoşkun, O.-
dc.contributor.authorKumtepe, A.-
dc.contributor.authorKaragöz, E.-
dc.contributor.authorSankır, Mehmet-
dc.contributor.authorDemirci Sankır, Nurdan-
dc.date.accessioned2021-01-27T13:24:31Z-
dc.date.available2021-01-27T13:24:31Z-
dc.date.issued2020-09
dc.identifier.citationTuc Altaf, C., Sahsuvar, N. S., Abdullayeva, N., Coskun, O., Kumtepe, A., Karagoz, E., ... and Demirci Sankir, N. (2020). Inverted Configuration of Cu (In, Ga) S2/In2S3 on 3D-ZnO/ZnSnO3 Bilayer System for Highly Efficient Photoelectrochemical Water Splitting. ACS Sustainable Chemistry and Engineering, 8(40), 15209-15222.en_US
dc.identifier.issn21680485
dc.identifier.urihttps://hdl.handle.net/20.500.11851/4105-
dc.identifier.urihttps://pubs.acs.org/doi/10.1021/acssuschemeng.0c04846-
dc.description.abstractIntroducing a zinc stannate, ZnSnO3 (ZTO), layer on hydrothermally grown 3D-zinc oxide (ZnO) nanosheet thin films has been proven to have a quenching effect on the photoluminescence emissions, indicating very slow recombination of photoinduced electron-hole pairs in photoelectrochemical water splitting (PEC) reactions. Motivated by this, the ZnO/ZTO bilayer system has been used as the electron transport layer for copper indium gallium sulfide (CIGS)-based photoelectrodes in PEC applications. Furthermore, the poor photoresistivity of CIGS has been improved via indium sulfide (In2S3) deposition. Consequently, the photoelectrode obtained from the inverted configuration, ZnO/ZTO/CIGS/In2S3, has generated a photocurrent density of 6.4 mA cm-2 at 0.4 V (vs Ag/AgCl), exceeding the performance of ZnO NS/CIGS/In2S3 photoelectrodes by three folds. The highest ABPE and IPCE efficiencies have been calculated as 4.2% and 57%, respectively. More importantly, two cost-effective nonvacuum techniques for large-scale thin film fabrications such as chemical bath deposition (CBD) and ultrasonic spray pyrolysis (USP) methods have been adopted to acquire photoelectrodes with inverted configurations providing an advantageous approach for low-cost photoelectrode design for sustainable energy production. Copyright © 2020 American Chemical Society.en_US
dc.language.isoenen_US
dc.publisherAmerican Chemical Societyen_US
dc.relation.ispartofACS Sustainable Chemistry and Engineeringen_US
dc.rightsinfo:eu-repo/semantics/closedAccessen_US
dc.subject3D-ZnOen_US
dc.subjectCopper indium gallium sulfideen_US
dc.subjectIndium sulfideen_US
dc.subjectPhotoelectrochemical water splittingen_US
dc.subjectSpray pyrolysisen_US
dc.subjectZnSnO3en_US
dc.titleInverted Configuration of Cu(In,Ga)S2/In2S3on 3D-ZnO/ZnSnO3Bilayer System for Highly Efficient Photoelectrochemical Water Splittingen_US
dc.typeArticleen_US
dc.departmentFaculties, Faculty of Engineering, Department of Material Science and Nanotechnology Engineeringen_US
dc.departmentFakülteler, Mühendislik Fakültesi, Malzeme Bilimi ve Nanoteknoloji Mühendisliği Bölümütr_TR
dc.identifier.volume8
dc.identifier.issue40
dc.identifier.startpage15209
dc.identifier.endpage15222
dc.relation.tubitakinfo:eu-repo/grantAgreement/TÜBİTAK/MAG/315M348en_US
dc.authorid0000-0002-7004-1217-
dc.authorid0000-0003-2103-0439-
dc.identifier.wosWOS:000579972900012en_US
dc.identifier.scopus2-s2.0-85094929763en_US
dc.institutionauthorSankır, Mehmet-
dc.institutionauthorDemirci Sankır, Nurdan-
dc.identifier.doi10.1021/acssuschemeng.0c04846-
dc.relation.publicationcategoryMakale - Ulusal Hakemli Dergi - Kurum Öğretim Elemanıen_US
item.cerifentitytypePublications-
item.grantfulltextnone-
item.openairetypeArticle-
item.openairecristypehttp://purl.org/coar/resource_type/c_18cf-
item.fulltextNo Fulltext-
item.languageiso639-1en-
crisitem.author.dept02.6. Department of Material Science and Nanotechnology Engineering-
crisitem.author.dept02.6. Department of Material Science and Nanotechnology Engineering-
Appears in Collections:Malzeme Bilimi ve Nanoteknoloji Mühendisliği Bölümü / Department of Material Science & Nanotechnology Engineering
Scopus İndeksli Yayınlar Koleksiyonu / Scopus Indexed Publications Collection
WoS İndeksli Yayınlar Koleksiyonu / WoS Indexed Publications Collection
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